Synthesis of CZTS kesterite by pH adjustment in order to improve the performance of CZTS thin film for photovoltaic applications
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| dc.contributor.author | Aamir Shafi, Muhammad
|
es_ES |
| dc.contributor.author | Khan, Laiq
|
es_ES |
| dc.contributor.author | Ullah, Shafi
|
es_ES |
| dc.contributor.author | Bouich, Amal
|
es_ES |
| dc.contributor.author | Ullah, Hanif
|
es_ES |
| dc.contributor.author | Mari, Bernabé
|
es_ES |
| dc.date.accessioned | 2024-04-24T18:06:19Z | |
| dc.date.available | 2024-04-24T18:06:19Z | |
| dc.date.issued | 2022-04 | es_ES |
| dc.identifier.issn | 0749-6036 | es_ES |
| dc.identifier.uri | http://hdl.handle.net/10251/203727 | |
| dc.description.abstract | [EN] Quaternary CZTS (Cu2ZnSnS4) kesterite thin layers were successfully made by electrochemical deposition method. CZTS thin layers were deposited on Indium Tin Oxide (ITO) from an aqueous solution. In this work, the effects of pH adjustment under ambient conditions of CZTS thin films were studied. The as grown samples were investigated by numerous existing characterization systems. The X-ray diffraction (XRD) proves the polycrystalline description of the layer. The average crystallite size is varying from 10 nm to 24 nm of the films is dependent on the pH of the solution. All the thin films are in the CZTS kesterite phase attributed to A(1) mode at 334 cm(-1) verified by Raman spectroscopy. The SEM and AFM study show that the pH variation of the so-lution improved the surface morphology and topography of the CZTS thin films which increase several nm in grain size. Moreover, the optical analysis indicates a suitable band gap in the range of 1.5-1.8 eV depending upon the sulfurization temperature. It is found that the pH variation affects both the stability and the performance of the high-quality CZTS absorber layer applications. The CZTS layer with 4.80 pH was annealed at 450 degrees C and 500 degrees C, and at these temperatures the band gap was varied. At the end the band gap variations effect on the performance of CZTS based solar cell is being analyzed by using a simulation tool SCAPS-1D. | es_ES |
| dc.description.sponsorship | Author Sha fi Ullah acknowledged the post -doctoral contract supported by the, RRHH, postdoctoral contract (PAID-10-20), and Ministerio de Economia y Competitividad (Grant Number PID2019-107137RB-C21) , Universitat Politècnica de València (UPV) Spain. Author Amal Bouich acknowledged the Post -doctoral contract supported by the, RRHH, Postdoctoral contract the Margarita Salas fi nanced with union European Next Generation EU. This research has been funded by Grant PID2019-107137RB-C21 funded by MCIN/AEI/10.13039/501100011033 and by "ERDF A way of making Europe". The author Muhammad Aamir Sha fi acknowledge the Higher Education Commission of Pakistan, International Research Support Initiative Program (IRSIP) , for grant No: 1-8/HEC/HRD/2020/10744 PIN: IRSIP 45 Engg 17. | es_ES |
| dc.language | Inglés | es_ES |
| dc.publisher | Elsevier | es_ES |
| dc.relation.ispartof | Superlattices and Microstructures | es_ES |
| dc.rights | Reserva de todos los derechos | es_ES |
| dc.subject | CZTS | es_ES |
| dc.subject | PH adjustment | es_ES |
| dc.subject | Electrodeposition | es_ES |
| dc.subject | XRD | es_ES |
| dc.subject | Raman and optical Properties | es_ES |
| dc.subject.classification | FISICA APLICADA | es_ES |
| dc.title | Synthesis of CZTS kesterite by pH adjustment in order to improve the performance of CZTS thin film for photovoltaic applications | es_ES |
| dc.type | Artículo | es_ES |
| dc.identifier.doi | 10.1016/j.spmi.2022.107185 | es_ES |
| dc.relation.projectID | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PID2019-107137RB-C21/ES/MEJORANDO LA PRODUCCION DE ENERGIA SOLAR CON PEROVSKITAS INORGANICAS.SINTESIS/ | es_ES |
| dc.relation.projectID | info:eu-repo/grantAgreement/UNIVERSIDAD POLITECNICA DE VALENCIA//MS%2F27//AYUDA MARGARITA SALAS DE BOUICH, AMAL/ | es_ES |
| dc.relation.projectID | info:eu-repo/grantAgreement/UPV//PAID-10-20//SINTESIS Y CARACTERIZACIÓN DE SEMICONDUCTORES V: SnS2 CON BANDA INTERMEDIA PARA APLICACIONES FOTOCATALITICS Y FOTOVOLTAICAS AVANZADAS / | es_ES |
| dc.relation.projectID | info:eu-repo/grantAgreement/HEC//1-8%2FHEC%2FHRD%2F2020%2F10744/ | es_ES |
| dc.rights.accessRights | Cerrado | es_ES |
| dc.contributor.affiliation | Universitat Politècnica de València. Escuela Técnica Superior de Ingeniería del Diseño - Escola Tècnica Superior d'Enginyeria del Disseny | es_ES |
| dc.contributor.affiliation | Universitat Politècnica de València. Instituto de Diseño para la Fabricación y Producción Automatizada - Institut de Disseny per a la Fabricació i Producció Automatitzada | es_ES |
| dc.description.bibliographicCitation | Aamir Shafi, M.; Khan, L.; Ullah, S.; Bouich, A.; Ullah, H.; Mari, B. (2022). Synthesis of CZTS kesterite by pH adjustment in order to improve the performance of CZTS thin film for photovoltaic applications. Superlattices and Microstructures. 164:1-10. https://doi.org/10.1016/j.spmi.2022.107185 | es_ES |
| dc.description.accrualMethod | S | es_ES |
| dc.relation.publisherversion | https://doi.org/10.1016/j.spmi.2022.107185 | es_ES |
| dc.description.upvformatpinicio | 1 | es_ES |
| dc.description.upvformatpfin | 10 | es_ES |
| dc.type.version | info:eu-repo/semantics/publishedVersion | es_ES |
| dc.description.volume | 164 | es_ES |
| dc.relation.pasarela | S\457209 | es_ES |
| dc.contributor.funder | European Commission | es_ES |
| dc.contributor.funder | Agencia Estatal de Investigación | es_ES |
| dc.contributor.funder | European Regional Development Fund | es_ES |
| dc.contributor.funder | UNIVERSIDAD POLITECNICA DE VALENCIA | es_ES |
| dc.contributor.funder | Higher Education Commission, Pakistan | es_ES |
| dc.contributor.funder | Universitat Politècnica de València | es_ES |
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