One-pot chemo- and photo-enzymatic linear cascade processes
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| dc.contributor.author | Carceller-Carceller, Jose Miguel
|
es_ES |
| dc.contributor.author | Arias, Karen S.
|
es_ES |
| dc.contributor.author | Climent Olmedo, María José
|
es_ES |
| dc.contributor.author | Iborra Chornet, Sara
|
es_ES |
| dc.contributor.author | Corma Canós, Avelino
|
es_ES |
| dc.date.accessioned | 2025-02-27T13:49:58Z | |
| dc.date.available | 2025-02-27T13:49:58Z | |
| dc.date.issued | 2024-07-29 | es_ES |
| dc.identifier.issn | 0306-0012 | es_ES |
| dc.identifier.uri | http://hdl.handle.net/10251/214888 | |
| dc.description.abstract | [EN] The combination of chemo- and photocatalyses with biocatalysis, which couples the flexible reactivity of the photo- and chemocatalysts with the highly selective and environmentally friendly nature of enzymes in one-pot linear cascades, represents a powerful tool in organic synthesis. However, the combination of photo-, chemo- and biocatalysts in one-pot is challenging because the optimal operating conditions of the involved catalyst types may be rather different, and the different stabilities of catalysts and their mutual deactivation are additional problems often encountered in one-pot cascade processes. This review explores a large number of transformations and approaches adopted for combining enzymes and chemo- and photocatalytic processes in a successful way to achieve valuable chemicals and valorisation of biomass. Moreover, the strategies for solving incompatibility issues in chemo-enzymatic reactions are analysed, introducing recent examples of the application of non-conventional solvents, enzyme-metal hybrid catalysts, and spatial compartmentalization strategies to implement chemo-enzymatic cascade processes. This review explores linear cascade reactions by combining chemo-, photo- and biocatalysts for organic synthesis and strategies to overcome incompatibility issues. | es_ES |
| dc.description.sponsorship | This work has been funded by the Spanish Ministry of Science and Innovation through the "Severo Ochoa Program" (CEX-2021-001230-S) and the PID2021-125897OB-I00 (MCIU/AEI/) 10.13039/501100011033 by "ERDF A way of making Europe" project. J. M. C. thanks the Margarita Salas grant from the Ministerio de Universidades, Universitat Politecnica de Valencia, Spain, funded by the European Union-Next Generation EU (2021-2023). | es_ES |
| dc.language | Inglés | es_ES |
| dc.publisher | The Royal Society of Chemistry | es_ES |
| dc.relation.ispartof | Chemical Society Reviews | es_ES |
| dc.rights | Reconocimiento - No comercial (by-nc) | es_ES |
| dc.subject | Chemocatalyses | es_ES |
| dc.subject | Photocatalyses | es_ES |
| dc.subject | Biocatalysis | es_ES |
| dc.subject | Linear cascade processes | es_ES |
| dc.subject.classification | QUIMICA ORGANICA | es_ES |
| dc.title | One-pot chemo- and photo-enzymatic linear cascade processes | es_ES |
| dc.type | Artículo | es_ES |
| dc.type | Artículo de revisión | |
| dc.identifier.doi | 10.1039/D3CS00595J | es_ES |
| dc.relation.projectID | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/PID2021-125897OB-I00/ES/PROCESOS CATALITICOS AVANZADOS EN BIORREFINERIA PARA LA PRODUCCION DE COMBUSTIBLES Y PRODUCTOS QUIMICOS RENOVABLES/ | es_ES |
| dc.relation.projectID | info:eu-repo/grantAgreement/AEI//CEX2021-001230-S/ | es_ES |
| dc.rights.accessRights | Abierto | es_ES |
| dc.contributor.affiliation | Universitat Politècnica de València. Escuela Técnica Superior de Ingenieros Industriales - Escola Tècnica Superior d'Enginyers Industrials | es_ES |
| dc.description.bibliographicCitation | Carceller-Carceller, JM.; Arias, KS.; Climent Olmedo, MJ.; Iborra Chornet, S.; Corma Canós, A. (2024). One-pot chemo- and photo-enzymatic linear cascade processes. Chemical Society Reviews. 53(15):7875-7938. https://doi.org/10.1039/D3CS00595J | es_ES |
| dc.description.accrualMethod | S | es_ES |
| dc.relation.publisherversion | https://doi.org/10.1039/D3CS00595J | es_ES |
| dc.description.upvformatpinicio | 7875 | es_ES |
| dc.description.upvformatpfin | 7938 | es_ES |
| dc.type.version | info:eu-repo/semantics/publishedVersion | es_ES |
| dc.description.volume | 53 | es_ES |
| dc.description.issue | 15 | es_ES |
| dc.identifier.pmid | 38965865 | es_ES |
| dc.relation.pasarela | S\523399 | es_ES |
| dc.contributor.funder | Agencia Estatal de Investigación | es_ES |
| dc.contributor.funder | European Regional Development Fund | es_ES |
| dc.contributor.funder | Universitat Politècnica de València | es_ES |
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